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Previous examples of asymmetric three-component intermolecular alkene aminoarylations to attain - arylethylamines 38, 39. Reactions are limited to the utilization of a single class of terminal olefins, either styrenes (R1 = Ar) or vinyl amides (R1 = NHCOR), and thus to the generation of a single stereogenic centre. N -fluoro- N -methylsulfonamides (NFAS) and O -acyl hydroxylmethylamine were used as N-atom donors, providing access exclusively to N -Me tertiary amine products.
#Workflow#Flowchart#Illustration#Chemical Structure#Asymmetric three-component intermolecular alkene aminoarylations#Beta-arylethylamines#Olefins#Styrenes#Vinyl amides#N-fluoro- N -methylsulfonamides#O -acyl hydroxylmethylamine#N -Me tertiary amine products
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