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Open access visualization of Heatmap, fs-TAS, [2]Grid, Benzonitrile, Heat map
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fs-TAS of [2]Grid in argon-saturated benzonitrile. Left: heat map of fs-TAS raw data obtained at 530 nm photoexcitation with time delays up to 5500 ps. Right: evolution-associated spectra showing the singlet excited state (S1) (black), the relaxed singlet excited state mixing with charge transfer (S1)relCT(red), and symmetry-broken charge-separated state SB-CS (blue). Right: Respective population kinetics. Note that SB-CS is not completely deconvoluted on this time scale.

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