Line Plot from Scientific Research

Evolution of the OBF motion, characterized via the H-C=C-H dihedral angle as a geometric parameter. Shown are the 66 trajectories populating the T1state within 500 fs. The time evolution of OBF motion is synchronized with respect to entry into the T1state. Trajectories were extended for an additional 500 fs after population of the T1. The color scheme characterizes each individual trajectory according to the sign of the dihedral at the end of the simulation time. Interconversion between the faces was a rare event (two instances) and short-lived.

DOI